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張博凱 教授-兼課務組組長

張博凱 教授 兼課務組組長
Bor-Kae Chang
|                美國加州大學柏克萊化學工程學系/核能工程學系 雙學士
|                德國慕尼黑/奧格斯堡先進材料科學課程 碩士
|                英國劍橋大學材料科學系 博士
分機: 34236
辦公室: 工程四館 E3-301
研究室: 工程四館 E3-301
實驗室: 多孔性材料實驗室
Email: BKChang@ncu.edu.tw
“張博凱教授照片"

研究領域

金屬有機骨架材料、氣體分離薄膜、多尺度模擬、第一原理計算(density functional theory)。

多孔性材料在化工領域及工業用途有很重要的應用，包括氣體吸附、分離、以及儲存。新興材料，如金屬有機骨架材料(metal-organic frameworks, MOFs)以及沸石咪唑骨架材料(zeolitic imidazolate frameworks, ZIFs)等，因為組合單位選擇多、合成結構變化廣，以至於無法系統性地尋找合適的材料組合。透過合成分析以及第一原理模擬的配合，可以加速理解新開發之多孔性材料對於氣體的反應。 目前實驗室的研究題目包括:

• MOF、ZIF材料合成及應用

• 薄膜製作及氣體分離測試

• 材料與氣體反應之第一原理計算 (density-functional theory, DFT)

活動照片1

論文著作

  1. Wu, C.-Y., Chang, B.K.,* “Effect of ZIF-78 metal-organic framework crystal morphology and defect in resulting polysulfone mixed matrix membranes”, J. Taiwan Inst. Chem. Eng., 2024, 157, 105418.
  2. Puspitasari, D.A., Patra, J., Hernandha, R.F.H., Chiang, Y.-S., Inoishi, A., Chang, B.K.,* Lee, T.-C.,* Chang, J.-K.,* “Enhanced Electrochemical Performance of Ca-Doped Na3V2(PO4)2F3/C Cathode Materials for Sodium-Ion Batteries”, ACS Appl. Mater. Interfaces, 2024, 16, 1, 496-506.
  3. Arshad, M.U., Dutta, D., Sin, Y.Y., Hsiao, S.W., Wu, C.Y., Chang, B.K., Dai, L., Su, C.Y., “Multi-functionalized fluorinated graphene composite coating for achieving durable electronics: Ultralow corrosion rate and high electrical insulating passivation”, Carbon, 2022, 195, 141-153.
  4. Zhuang, S.-H., Yang, C.-C., Zheng, M., Rengapillai, S., Marimuthu, S., Chiang, Y.-S., Chang, B.K., Liu, W.-R., “A combined first principles and experimental study on Al-doped Na3V2(PO4)2F3 cathode for rechargeable Na batteries”, Surf. Coat. Technol., 2022, 434, 128184.
  5. Muruganantham, R., Lin, M.-C., Wang, P.K., Chang, B.K., Liu, W.-R., “Highly effective Al-doped titanium niobate porous anode material for rechargeable high-rate Li-ion storage performance”, J. Taiwan Inst. Chem. Eng., 2022 131, 104187.
  6. Huang, G., Ghalei, B., Isfahani, A.P., Karahan, H.E., Terada, D., Qin, D., Li, C., Tsujimoto, M., Yamaguchi, D., Sugimoto, K., Igarashi, R., Chang, B.K., Li, T., Shirakawa, M., Sivaniah, E., "Overcoming humidity-induced swelling of graphene oxide-based hydrogen membranes using charge-compensating nanodiamonds", Nature Energy, 2021, 6, 1176-1187.
  7. Wu, K.-C., Chieh, C.-M.,* Chang, B.K.,* "First principles calculations on lithium diffusion near surface and in bluk of Fe-doped LiCoPO4", Physical Chemistry Chemical Physics, 2021, DOI: 10.1039/D1CP04517B.
  8. Kao, S.-N., Hung, Y.-C., Shimoyama, Y., Hsieh, C.-M.,* Chang, B.K.,* "Investigating lithium intercalation and diffusion in Nb-doped TiO2 by first principles calculations", Journal of the Taiwan Institute of Chemical Engineers, 2021, 125, 314-322.
  9. Patra, J., Wu, S.-C., Leu, I.-C., Yang, C.-C., Dhaka, R.S., Okada, S., Yeh, H.-L., Hsieh, C.-M., Chang, B.K.,* Chang, J.-K.,* "Hydrogenated Anatase and Rutile TiO2 for Sodium-Ion Battery Anodes", ACS Applied Energy Materials, 2021, 4, 6, 5738-5746.
  10. Chan, S.-C., Cheng, Y.-L., Chang, B.K.,* Hong, C.-W.,* "The origins of charge separation in anisotropic facet photocatalysts investigated through first-principles calculations", RSC Advances, 2021, 11, 18500-18508.
  11. Ou, J.-H., Sheu, Y.-T., Chang, B.K., Verpoort, F., R.Y. Surampalli, Kao, C.-M., "Application of zeolitic imidazolate framework for hexavalent chromium removal: A feasibility and mechanism study", Water Environment Research, 2021: doi.org/10.1002/wer.1571.
  12. Wu, X.-M., Chang, B.K.,* Hsieh, C.-M.,* "Computational study on the effect of steric hindrance in functionalised Zr-based metal-organic frameworks on hydrocarbon storage and separation", Molecular Simulation, 2021, 47, 7, 565-574.
  13. Yuan, S.H., Isfahani, A.P., Yamamoto, T., Muchtar, A., Wu, C.Y., Huang, G., You, Y.C., Sivaniah, E., Chang, B.K., Ghalei, B., "Nanosized Core–Shell Zeolitic Imidazolate Frameworks‐Based Membranes for Gas Separation", Small Methods, 2020, 4, 8, 200021.
  14. Chao, C.-H., Ni, W.-C., Chen, C.-T., Chang, B.K., Huang, C.-H., Su, C.-Y., Liu, W.-R., "Synthesis, luminescence properties and theoretical calculations of La5BSi2O13:Dy3+ phosphor coatings for light-emitting diodes", Thin Solid Films, 2020, 698, 137865.
  15. Muruganantham, R., Lu, J.-S., Maggay, I.V.B., Chang, B.K., Wang, P.K., Liu, W.-R., "Modification of spinel-based CoV2O4 materials through Mn substitution as a potential anode material for Li-ion storage", Surf. Coat. Technol., 2020, 389, 125602.

  16. Gesesse, G.D., Wang, C., Chang, B.K., Tai, S.-H., Beaunier, P., Wojcieszak, R., Remita, H., Colbeau-Justin, C., Ghazzal, M.N., "A soft-chemistry assisted strong metal-support interaction on a designed plasmonic core-shell photocatalyst for enhanced photocatalytic hydrogen production", Nanoscale, 2020, 12, 7011-7023.

  17. Ghalei, B., Wakimoto, K., Wu, C.Y., Isfahani, A.P., Yamamoto, T., Sakurai, K., Higuchi, M., Chang, B.K., Kitagawa, S., Sivaniah, E., "Rational Tuning of Zirconium Metal-Organic Framework Membranes for Hydrogen Purification", Angew. Chemie Int. Ed., 2019, 58, 52, 19034-19040.
  18. Tai, S.-Y., Muruganantham, R., Tai, S.-H., Chang, B.K., Wu, S.-C., Chueh, Y.-L., Liu, W.-R., “Coffee grounds-derived carbon as high performance anode materials for energy storage applications”, J. Taiwan Inst. Chem. Eng., 2019, 97, 178-188.
  19. Tran, B.-L., Chin, H.-Y., Chang, B.K.,* Chiang, A.S.T.,* “Dye Adsorption in ZIF-8: The Importance of External Surface Area”, Microporous Mesoporous Mater., 2019, 277, 149-153.
  20. Tai, S.-H., Chang, B.K.,* “Effect of nitrogen-doping configuration in graphene on the oxygen reduction reaction”, RSC Adv., 2019, 9, 6035-6041.
  21. Liao, C.-W., Tseng, P.-S., Chang, B.K., Wang, C.-Y., “Facilitated Hydrogen Release Kinetics from Amine Borane Functionalization on Gate-Opening Metal-Organic Framework”, Surf. Coat. Technol., 2018, 350, 12-19.
  22. Chang, Y.-W., Chang, B.K.,* “Influence of casting solvents on sedimentation and performance in metal–organic framework mixed-matrix membranes”, J. Taiwan Inst. Chem. Eng., 2018, 89, 224-233.
  23. Yeh, H.-L., Tai, S.-H., Hsieh, C.-M.,* Chang, B.K.,* “First-Principles Study of Lithium Intercalation and Diffusion in Oxygen-Defective Titanium Dioxide”, J. Phys. Chem. C, 2018, 122(34), 19447-19454.
  24. Maggay, I.V.B., De Juan, L.M.Z., Nguyen, M.T., Yonezawa, T., Chang, B.K., Chan, T.S., Liu, W.-R., “ZnV2O4: A Potential Anode Material for Sodium-Ion Batteries”, J. Taiwan Inst. Chem. Eng., 2018, 88, 161-168.
  25. Chung, J.-Y., Liao, C.-W., Chang, Y.-W., Chang, B.K., Wang, H., Li, J., Wang, C.-Y., “Influence of Metal-Organic Framework Porosity on Hydrogen Generation from Nanoconfined Ammonia Borane”, J. Phys. Chem. C, 2017, 121(49), 27369-27378.
  26. Hao, S.-W., Hsu, C.-H., Liu, Y.-G., Chang, B.K.,* “Activated Carbon Derived from Hydrothermal Treatment of Sucrose and Its Air Filtration Application”, RSC Adv., 2016, 6, 109950-109959.
  27. Chang, H.-L., Chen, C.-M., Lin, K.-L., Chang, B.K., “Study on the Effects of Diluent on Silica/Epoxy Resin Composite Material Phase Change”, Appl. Mech. Mater., 2014, 459, 34-39.
  28. Chang, H.-L., Chen, C.-M., Lin, K.-L., Chang, B.K., “The Effects of Chemical Resistance for Nanocomposite Materials via Nano-Silica Addition into Glass Fiber/Epoxy”, Adv. Mat. Res., 2014, 853, 28-33.
  29. Chang, B.K.,* Bristowe, P.D. & Cheetham, A.K., “Computational Studies on the Adsorption of CO2 in the Flexible Perfluorinated Metal-Organic Framework Zinc 1,2-bis(4-pyridyl)ethane tetrafluoroterephthalate”, Phys. Chem. Chem. Phys., 2013, 15, 176-182.
  30. Chang, B.K.,* Bristowe, N.C., Bristowe, P.D. & Cheetham, A.K., “Van der Waals Forces in the Perfluorinated Metal-Organic Framework Zinc 1,2-bis(4-pyridyl)ethane Tetrafluoroterephthalate”, Phys. Chem. Chem. Phys., 2012, 14, 7059-7064.